The correlations between flow harmonics $v_n$ for $n=2$, 3 and 4 and mean transverse momentum $[p_\mathrm{T}]$ in $^{129}$Xe+$^{129}$Xe and $^{208}$Pb+$^{208}$Pb collisions at $\sqrt{s_{\mathrm{NN}}}=5.44$ TeV and 5.02 TeV, respectively, are measured using charged particles with the ATLAS detector. The correlations are sensitive to the shape and size of the initial geometry, nuclear deformation, and initial momentum anisotropy. The effects from non-flow and centrality fluctuations are minimized, respectively, via a subevent cumulant method and event activity selection based on particle production in the very forward rapidity. The results show strong dependences on centrality, harmonic number $n$, $p_{\mathrm{T}}$ and pseudorapidity range. Current models describe qualitatively the overall centrality- and system-dependent trends but fail to quantitatively reproduce all the data. In the central collisions, where models generally show good agreement, the $v_2$-$[p_\mathrm{T}]$ correlations are sensitive to the triaxiality of the quadruple deformation. The comparison of model to the Pb+Pb and Xe+Xe data suggests that the $^{129}$Xe nucleus is a highly deformed triaxial ellipsoid that is neither a prolate nor an oblate shape. This provides strong evidence for a triaxial deformation of $^{129}$Xe nucleus using high-energy heavy-ion collision.
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